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I was using PyQt5/PySide which will give you a nice native look but I eventually shifted over to DearPyGui for most of my smaller utilities. Its just faster for me. You will get more options and freedom with PyQt/PySide though and can use QT Designer to design your interfaces pretty easily.
We just rolled out an internal application using NiceGUI, and it looks and works great. Highly recommend!
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The number of mentions on this list indicates mentions on common posts plus user suggested alternatives.
Hence, a higher number means a more popular project.