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I would stick with pySimpleGui until you find a requirement that it can't fulfill. At least skinning should be possible, see for example https://github.com/PySimpleGUI/PySimpleGUI/issues/3412 with loads of examples.
Dear PyGui is a GUI framework that seems to be increasingly popular with engineers and scientists. Obviously, it depends on your requirements. PyQt/Pyside and Electron are probably the most mature libraries with their own strengths. Potential downside to PyQt/Pyside is the license. Electron GUI is most like the web. Downside is the library size as it basically includes Chromium.